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Spectral properties of an efficient entangled photon source based on bulk PPKTP

Abstract

English: The main objective of this thesis is to study and characterize the spectral properties of spontaneous parametric down conversion (SPDC) generated in bulk periodically poled potassium titanyl phosphate (PPKTP). The work carried out is an essential step towards the implementation of a high brigthness photon-pair source for long distance quantum key distribution (QKD) experiments in a free-space environment.

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Spectral properties of an efficient entangled photon source based on bulk PPKTP

Author: Pérez Gumà, Daniel
Publisher: Universitat Politècnica de Catalunya
Year: 2011
Source: https://upcommons.upc.edu/bitstream/2099.1/12996/1/Master_Thesis_ICFO_-_Final_Document_-_Daniel_Perez.pdf
MSc in Pho onics PHOTONICSBCN
Uni e si a Poli ècnica de Ca alunya (UPC)
Uni e si a Au ònoma de Ba celona (UAB)
Uni e si a de Ba celona (UB)
Ins i u de Ciències Fo òniques (ICFO)
h p://www.pho onicsbcn.eu
Mas e in Pho onics
MASTER THESIS WORK
SPECTRAL PROPERTIES OF AN EFFICIENT
ENTANGLED PHOTON SOURCE BASED ON
BULK PPKTP
Daniel Pé ez Gumà
Supe ised by D . Vale io P une i, (ICFO)
P esen ed on da e 1s Sep embe 2011
Regis e ed a
Spec al p ope ies o an e icien en angled pho on
sou ce based on bulk PPKTP
Daniel P´e ez Gum`a
ICFO - Ins i u de Ci`encies Fo `oniques, Medi e anean Technology Pa k, 08860
Cas ellde els (Ba celona), Spain
E-mail: [email p o ec ed]
Abs ac . The main objec i e o his hesis is o s udy and cha ac e ize he spec al
p ope ies o spon aneous pa ame ic down con e sion (SPDC) gene a ed in bulk
pe iodically poled po assium i anyl phospha e (PPKTP). The wo k ca ied ou
is an essen ial s ep owa ds he implemen a ion o a high b ig hness pho on-pai
sou ce o long dis ance quan um key dis ibu ion (QKD) expe imen s in a ee-space
en i onmen .
Keywo ds. Quan um key dis ibu ion,spon aneous pa ame ic down con e sion,PPKTP
1. In oduc ion and mo i a ion
Nowadays socie y needs o as and secu e communica ions is undeniable. Up o
he p esen ime communica ion and c yp og aphy echniques a e being used aking
ad an age o ou knowledge abou he ealm o classical physics. In his con ex classical
elec odynamics is he solid g ound in which all cu en communica ion sys ems a e
based: wi i local a ea ne wo ks, mobile communica ions, op ical ne wo ks, blue oo h,
e c. . . Howe e , quan um physics has become an in ensi ely s udied esea ch ield o e
he las cen u y. I u ns ou some scien i ic and echnological b eak h oughs sugges
ha cu en classical c yp og aphy could be de ea ed by nea - u u e quan um sys ems.
This is he eason why he scien i ic communi y is pu suing he c ea ion o quan um
communica ion sys ems.
1.1. The end o classical c yp og aphy
Classical c yp og aphy su e s om wo main laws: ei he he secu i y o a p o ocol is
no uncondi ional (i.e. 100% secu e) o he key exchange be ween he pa ies is e y
unp ac ical.
The i s issue is usually ela ed o public-key sys ems, whe e he secu i y o he
key is based on wha is called a one way unc ion. One-way unc ions a e ma hema ical
ope a ions ha a e e y easy o compu e in one way, bu e y di icul o e e se.
Spec al p ope ies o an e icien en angled pho on sou ce based on bulk PPKTP 2
An example o his echnique is he widely used RSA p o ocol whe e he secu i y is
based on he di icul y o inding he p ime ac o s o la ge in ege s. Finding he p ime
ac o s o a numbe using a classical compu e is a p oblem ha has exponen ially
g owing complexi y wi h espec o he key leng h. Howe e , i has been demons a ed
ha he e exis s a leas one ou ine (Sho ’s algo i hm) implemen able in a quan um
compu e ha can sol e his one-way unc ion in polynomial ime. The e o e, he pa h
owa ds quan um compu a ion ende s classical public-key sys ems.
The second issue is usually ela ed o sec e -key sys ems. In his case he secu i y
o he da a is based on he assump ion ha only he wo pa ies in ol ed know he
key. This is e y unp ac ical because one en i y migh wan o exchange in o ma ion
secu ely wi h many pa ies, he e o e needing many di e en keys. Mo eo e , only he
ace- o- ace key exchange would be 100% secu e, which is expensi e and ime consuming.
QKD can sol e he p oblems men ioned be o e. Thanks o he laws o quan um
mechanics, he secu i y o he keys is assu ed and hei c ea ion is emo ely nego ia ed.
Quan um p o ocols a e based on he exchange o quan um pa icles be ween he wo
pa ies namely Alice and Bob. A se ies o measu emen s o he s a es o such pa icles
by Alice and Bob enable he c ea ion o he secu e key [2].
1.2. Ou line o he p ojec
In sec ion 2 he design o he en angled pho on sou ce is desc ibed. The nume ical model
and i s main pa ame e s a e commen ed as well. In sec ion 3 he expe imen al se -up
is shown and discussed. Finally in sec ion 4 he esul s ob ained in he labo a o y a e
analyzed and compa ed wi h he nume ical model.
2. Theo y
Cu en ly, SPDC is he mos widely used physical p ocess o c ea e en angled pho on
pai s. This phenomenon is pu ely quan um, aking place a he pa icle le el. SPDC
can be unde s ood as a spon aneous decay o one pho on a eling in a nonlinea op ical
medium in o a pai o lowe ene gy pho ons called signal and idle . The p ocess is
allowed only when ene gy and momen um a e conse ed. The ene gy conse a ion can
be exp essed in e ms o he pho on ene gy as
¯hωp= ¯hωs+ ¯hωi(1)
whe e ωp,s,i is he angula equency o he pump, signal and idle pho ons
espec i ely. The echnique aiming a achie ing momen um conse a ion is called phase
ma ching. The e a e wo app oaches ha can ul ill he momen um conse a ion law:
bi e ingence and quasi phase ma ching (QPM). In his p ojec he QPM app oach has
been chosen mainly because o wo ad an ages wi h espec he bi e ingence echnique.
Fi s , he highes nonlinea coe icien o he c ys al can be used (in ou c ys al we
will exploi d33). Secondly, aligning he di ec ion o p opaga ion wi h one o he
c ys allog aphic axes, he beam does no su e he walk-o e ec because he wa e ec o
Spec al p ope ies o an e icien en angled pho on sou ce based on bulk PPKTP 3
and he poyn ing ec o a e pa allel. The e o e, he beam is be e con ined and as a
consequence he nonlinea in e ac ion is mo e e icien .
The QPM is achie ed in ou case by means o a e oelec ic pe iodic poling
echnique o he PPKTP c ys al. The pe iodically e e sed c ys allog aphic axes
o ien a ion enables he phase misma ch compensa ion be ween he pump, signal and
idle . The domain in e sion is enginee ed applying s ong elec ic ields by means o
pa e ned elec odes. The ini ial design o he pho on sou ce de e mined a alue o
3.425µm o he poling pe iod.
The pe iodically poled c ys al s uc u e has he key ole in he momen um
conse a ion equa ion. The phase ma ching condi ion o a collinea in e ac ion can
be w i en as [3]
kp=ks+ki+2π
Λ(2)
whe e kp,s,i a e he pump, signal and idle momen a and Λ is he poling pe iod o
he PPKTP c ys al. The e o e, he momen a misma ch can be exp essed as
∆k= 2π np(λp, T)
λp
−ns(λs, T)
λs
−ni(λi, T)
λi
−1
Λ!(3)
whe e he dependence o he e ac i e indices np,s,i wi h espec o he wa eleng h
and he empe a u e ha e been w i en. Using a con inuous wa e (CW) pump, he
spec um o he SPDC is [1]
S(λs,i)∝sinc2∆kL
2(4)
whe e Lis he leng h o he PPKTP c ys al, and ∆kis he exp ession (3). The
SPDC p ocess in ou expe imen s co esponds o ype 0 (pump,signal and idle ha e
he pola iza ion along he zaxis o he c ys al).
En anglemen is c ea ed by c ossing he c ys allog aphic z-axis o wo iden ical
PPKTP c ys als a 90 deg ees wi h espec o each o he . Signal and idle om he i s
and second c ys als a e supe posed and he elec ic ield can be w i en as a quan um
supe posi ion o bo h con ibu ions, ha ing o hogonal pola iza ions due o he c ys al
o ien a ions. The mos gene al o m o he quan um s a e gene a ed in his con igu a ion
may be w i en as
|Hsi ⊗ |Hii+eiφ |Vsi ⊗ |Vii(5)
whe e Hand Vs and o he ho izon al and e ical pola iza ions, and he
subindices e e o signal o idle wa eleng hs. The phase φcan be con olled o p oduce
di e en Bell s a es. The quali y o he en anglemen depends on he indis inguishabli y
o he ield coming om he i s and he second c ys al. Any measu able p ope y being
di e en lowe s he amoun o en anglemen . Fo his eason, a igo ous cha ac e iza ion
o he SPDC spec a as well as compa ison wi h he model calcula ion will be p esen ed
in he ollowing.
Spec al p ope ies o an e icien en angled pho on sou ce based on bulk PPKTP 4
The nume ical model is an implemen a ion in MATLAB o he spec um p o ile o
SPDC shown in equa ion (4). The unknown pa ame e s needed o be ound in o de o
cha ac e ize he se -up a e he e ac i e index o he pump np(λp, T) and he e ec i e
leng h o he c ys als Le . In sec ion 4 he me hods ollowed o ind hese pa ame e s
a e de ailed.
3. Se -up
The expe imen al se -up is shown in igu e 1. Two di e en lase s we e ixed, one
being single-mode and he o he mul i-mode. The ligh is coupled in o single mode
ibe s (SMFs). The lase is selec ed connec ing he desi ed ibe wi h he launching ibe
(do ed-line ibe s indica e ha hey a e used o no depending on he expe imen ). The
pola iza ion o he pump is con olled wi h he qua e -wa e pla e (QWP) and he hal -
wa e pla e (HWP). The luo escence il e p e en s possible long-wa eleng h adia ion
o c oss he c ys al and each he a alanche pho odiodess (APDs). The ocusing lens
plus he collima ing lens enable o p ope ly ocus he pump beam inside he c ys al.
The pump cu il e plays he same ole as he luo escence il e , bu in his case he
pump beam is blocked. In bo h cases he goal is p o ec ing he APDs om high powe
adia ion. Finally he wa eleng h di ision mul iplexe (WDM) spli s he SPDC ield in
wo di e en ibe s, being one co esponding o he signal and he o he o he idle .
Fo he expe imen s in which he spec um o he SPDC is eco ded, he ligh is sen
di ec ly o a monoch oma o .
Figu e 1. Se -up o he expe imen s. Two di e en pumping lase s can be used, one
being single mode and he o he mul imode. The beam is p ope ly ocused inside he
PPKTP c ys al wi h a ocusing and collima ing lenses. Two di e en SPDC de ec ion
s ages a e used, one being he monoch oma o ( o spec al analysis) and he o he
he WDM plus he APDs ( o pho on coincidences analysis)

Spec al p ope ies o an e icien en angled pho on sou ce based on bulk PPKTP 5
4. Resul s
4.1. The mal and wa eleng h expansion o he e ac i e index o he pump
The sellmeie equa ions used [4] [5] in he nume ical model ha e p e iously been epo ed
o ha e limi ed applicabili y in he pump wa eleng h egion [6], and only apply o signal
and idle . Since he PPKTP is hea ed a di e en empe a u es inside he o en and
pumped wi h a mul imode lase , a he mal and wa eleng h expansions o he e ac i e
index a e needed o comple e he nume ical model. Fi s he 4 h o de wa eleng h
expansion is compu ed a a ixed empe a u e (50℃). The ixed wa eleng h a ound
which he polynomial expansion is calcula ed co esponds o he single mode lase cen e
wa eleng h: 405.42nm.
In igu e 2(a) he esul is shown. As i can be seen he cen e wa eleng hs o he
di e en modes ma ch, which alida es he polynomial exp ession ound. The spec al
ampli udes p o ided by he simula ion seem o be unp ecise. The eason is ha he
mul imode pump spec um has a noisy beha io which a ec s he empo al e olu ion
o he ampli udes o he modes. Since he spec um eco ding p ocess in ol es a ime
in eg a ion, he inal ampli ude has a andom componen .
(a) (b)
Figu e 2. (a) Mul imode spec al in ensi y o SPDC a 50℃used o compu e he
wa eleng h expansion o he e ac i e index (b) Mul imode pump spec um o he
wa eleng h expansion expe imen
Once he wa eleng h dependence o he index o e ac ion is known, he he mal
coe icien s a e compu ed. The me hod o do i consis s o ma ching he signal and
idle cen e wa eleng hs wi hin a su icien ly wide ange o empe a u es. The e e ence
empe a u e is 50℃because he wa eleng h expansion has been calcula ed a his alue.
The single mode lase is used his ime. The 2nd o de expansion p o ides a e y good
ag eemen be ween he simula ion and he expe imen al da a as i can be seen in igu e 3.
To check ha he he mal and wa eleng h expansion wo k ine oge he , a
mul imode SPDC spec um is eco ded expe imen ally and simula ed a 48.3℃. Figu e 4
con i ms a good ag eemen o he join expansion wi h he expe imen .
Spec al p ope ies o an e icien en angled pho on sou ce based on bulk PPKTP 6
Figu e 3. Expe imen ally obse ed cen e wa eleng hs o signal and idle pho ons as a
unc ion o empe a u e. Simula ed da a shown using he op imized he mal expansion
o he pump e ac i e index
Figu e 4. Mul imode SPDC spec um a 48.3℃o he 20mm PPKTP c ys al.
The cen e wa eleng hs o he mul iple peaks a e ma ched, he e o e his expe imen
alida es he he mal-wa eleng h join expansion o he index o e ac ion a he pump
wa eleng h egion.
The exp ession o he pump e ac i e index wi h he mal and wa eleng h
expansions can be inally w i en as
np(λ, T) = np(λ0, T0) + A(T−T0) + B(T−T0)2+C(λ−λ0) +
D(λ−λ0)2+E(λ−λ0)3+F(λ−λ0)4(6)
whe e T0= 50℃and λ0= 405.42nm.
4.2. Bandwid h
Ha ing analyzed he cen e wa eleng h o he peaks, he o he impo an pa ame e om
he communica ions poin o iew is he spec al ull wid h hal maximum (FWHM).
Spec al p ope ies o an e icien en angled pho on sou ce based on bulk PPKTP 7
Like he cen e wa eleng h, he FWHM is empe a u e dependen [1], bu also he leng h
o he c ys al de ines he bandwid h. The longe he c ys al he na owe he peaks.
F om expe imen s eco ded o di e en empe a u es we de e mined he e ec i e leng h
o he c ys als. The speci ica ions o he manu ac u e only assu e ha he e ec i e
leng h is highe han 90% o he physical leng h, bu do no p o ide he exac alues.
In igu e 5 he FWHM o signal and idle a e depic ed o he L= 6.2mm c ys al as a
unc ion o empe a u e. The simula ion ma ches he expe imen al esul s a almos all
empe a u es. Only o e y low empe a u es nea he degene acy poin he simula ion
p o ides sligh ly highe alues han he expe imen s. The e ec i e leng h ha p o ides
a be e i ing o he expe imen co esponds o 98% o he physical leng h.
Figu e 5. Expe imen al FWHM o signal and idle as a unc ion o he empe a u e
o he 6.2mm PPKTP c ys al. The e ec i e leng h ha be e i s he simula ion
wi h he expe imen al poin s co esponds o Le = 6.08 (98% o he physical leng h)
In [1] he esul o he heo e ical FWHM wi h espec o he c ys al leng h is
p o ided. I u ns ou he bandwid h o he signal/idle is in e sely p opo ional o he
c ys al leng h. A nume ical simula ion has been ca ied ou o check he ag eemen o
he expe imen al esul s wi h he nume ical model. In igu e 6 he FWHM dependency
wi h espec o he c ys al e ec i e leng h is shown a T= 50℃. Fo la ge c ys al
leng hs he non negligible 1.2nm esolu ion o he monoch oma o s masks he eal 1
L
dependence, and he expe imen ally eco ded FWHMs a e sligh ly highe han he alues
ob ained wi h heo y.
4.3. Angle de uning
Up o now he beha io o he sys em wi h espec o empe a u e, c ys al leng h and
pump wa eleng h ha e been analyzed. Ano he ole ance ha needs o be es ed is he
angle o incidence o he pump beam. The quali y o he op omechanics used o ix
he componen s ely on he ole ance o misalignmen s. To check his issue a sweep
o he angle o incidence o he pump has been pe o med. The cen e wa eleng h o
he idle peaks is shown in igu e 7. The highes cen e wa eleng h co esponds o
Spec al p ope ies o an e icien en angled pho on sou ce based on bulk PPKTP 8
Figu e 6. FWHM o signal and idle a 50℃in on o he e ec i e leng h o he
PPKTP c ys al. Expe imen al da a is shown o he 20mm c ys al (18mm e ec i e
leng h) and he 6.2mm c ys al (6.08mm e ec i e leng h).
no mal incidence, which means ha he poling pe iod seen by he beam co esponds
o he alue p o ided by he manu ac u e . When he incidence angle is de uned (bo h
posi i ely and nega i ely), he e ec i e poling pe iod inc eases and his modi ies he
QPM equa ion, o cing signal and idle o mo e apa as hey do when he empe a u e
o he c ys al is inc eased.
Figu e 7. Expe imen al cen e wa eleng h d i as a unc ion o he ho izon al angle
o incidence o he pump beam. This e ec is caused, as a i s app oxima ion, by he
inc ease o he e ec i e poling pe iod when he incidence o he pump is no no mal
o he inpu ace o he c ys al.
4.4. E iciency o he sou ce using a WDM
One o he in e es ing pa ame e s o he sou ce is he numbe o pho ons pe second
emi ed. The highes b igh ness (coincidences[MHz]/pump powe [mW]) eco ded du ing
he p ojec was 5.66MHz
mW , ha ing a spec al b ig hness (coincidences[MHz]/pump powe