Double charge-exchange reactions and the effect of transfer
Abstract
There is a recently renewed interest on the study of single and double charge exchange reactions with heavy ions. We report here a preliminary theoretical study of double charge exchange reactions in terms of two successive charge exchanges in 2nd order Distorted Wave Born approximation. This allows us to include the effect of the different transfer channels in an approximate way. Evidences show that the charge exchange process is dominant. The following one in importance is the combination of one single charge exchange, one neutron pick-up and one proton stripping. This particular process calls for further investigation.
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Double cha ge-exchange eac ions and he e ec o
ans e
J A Lay1,†, S Bu ello2, J I Bellone2,3, M Colonna2and H Lenske4
wi hin he NUMEN p ojec
1Dp o. de F´ısica A ´omica, Molecula y Nuclea , Uni e sidad de Se illa, Se illa, Spain
2Is i u o Nazionale di Fisica Nuclea e, Labo a o i Nazionali del Sud, Ca ania, I aly
3Dipa imen o di Fisica e As onomia, Uni e si di Ca ania, I aly
4Ins i u ¨u Theo e ische Physik, Uni e si y o Giessen, Giessen, Ge many
E-mail: †[email protected]
Abs ac . The e is a ecen ly enewed in e es on he s udy o single and double cha ge
exchange eac ions wi h hea y ions. We epo he e a p elimina y heo e ical s udy o double
cha ge exchange eac ions in e ms o wo successi e cha ge exchanges in 2nd o de Dis o ed
Wa e Bo n app oxima ion. This allows us o include he e ec o he di e en ans e channels
in an app oxima e way. E idences show ha he cha ge exchange p ocess is dominan . The
ollowing one in impo ance is he combina ion o one single cha ge exchange, one neu on
pick-up and one p o on s ipping. This pa icula p ocess calls o u he in es iga ion.
1. In oduc ion
Nuclea eac ions a e one o he mos impo an ools o un a el he na u e o he in e ac ion
be ween neu ons and p o ons inside he a omic nucleus. In p inciple, we can ex ac a lo o
in o ma ion by making collide a nucleus o in e es wi h a ligh ion o wi h a hea y ion. In
he la e case, he heo e ical desc ip ion o he eac ion is la gely mo e in ol ed, since we
ha e o deal wi h he nucleon-nucleon in e ac ion o wo di e en many-body sys ems. In spi e
o his ex a di icul y, we ind in he li e a u e di e en cases in which we ha e imp o e ou
unde s anding o ce ain p oblems hanks o pa icula cha ac e is ics no a ailable wi h ligh
nuclei. As an example, we can ci e he s udy o b eakup o halo nuclei unde ex eme elec ic
ields supplied by a hea y a ge [1] o he sea ch o he Gian Pai ing Resonance, whe e a la ge
Q- alue is needed and only eachable wi h a hea y p ojec ile [2].
Fo he case o cha ge exchange eac ions, we can s udy he single cha ge exchange (SCE)
in he nucleus o in e es wi h bo h ligh and hea y ions. Howe e , pe o ming double cha ge
exchange (DCE) wi h ligh ions p esen s ce ain di icul ies like dealing wi h he measu emen
and econs uc ion o he ajec o y o h ee di e en inal p ojec ile pa icles as we would
ha e wi h a ligh ion like 3He o . We can use hea y ions o a oid such p oblems since bo h
he a ge -like and p ojec ile-like p oduc s o he eac ions will be bound in mos o he cases.
In addi ion, he inal c oss sec ion o double cha ge exchange will depend on he Fe mi and
Gamow Telle esponse o bo h he nucleus o in e es ( he a ge ) and he hea y ion used as
expe imen al p obe in he eac ion. By choosing ca e ully a hea y ion wi h a la ge Fe mi o
Gamow Telle esponse, we can inc ease he inal c oss sec ion, helping o he ex ac ion o he
pa icula esponse o he nucleus o in e es .
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Nowadays, he e is a la ge expe imen al in e es on double cha ge-exchange eac ions wi h
hea y ions which has gi en o igin o di e en campaigns mainly a he adioac i e beam acili ies
o RCNP a Osaka and RIKEN in Japan [3, 4] and a he LNS-INFN o Ca ania in I aly
[5, 6]. The o me ones a e ocused on s udying he Gamow-Telle esponse o nuclei and in he
p oduc ion o exo ic nuclei h ough double cha ge exchange eac ions. The la e is de o ed o
he s udy o double cha ge-exchange eac ions in connec ion wi h he neu inoless double-be a
decay.
In he p esen con ibu ion we will ocus in one o he eac ions pe o med a he LNS-INFN:
15 MeV/A 18O p ojec iles impinging on a 40Ca a ge [5]. A e he double cha ge-exchange we
will measu e 18Ne and 40A in di e en s a es. He e, we do no conside any di ec p ocess leading
om he ini ial o he inal coun e pa s. This means ha he nucleus-nucleus in e ac ion canno
change wo cha ges ac ing only once. Such a possibili y is unde in es iga ion [7]. The e o e,
he double cha ge-exchange is p oduced by a pa o he e ec i e nucleus-nucleus in e ac ion
able o change one cha ge a a ime bu ac ing wice, hus being called a second o de p ocess.
The inal si ua ion can be eached also h ough di e en combina ions o neu on pick-
up, p o on s ipping, and single cha ge-exchange p ocesses. Any o hese so-called compe ing
p ocesses is o a highe o de han he double cha ge-exchange, so ha his la e p ocess should
domina e. None heless, a low bomba ding ene gies, he di e ences can be oo small o neglec
he con ibu ion o he compe ing p ocesses. In any case, i we manage o con ol hem we can
ha e access o a complemen a y s uc u e in o ma ion o he nucleus conside ed which can be
o g ea in e es when s udying double-be a decay candida es.
The s udy o he compe i ion be ween cha ge exchange wi h hea y ion and he co esponding
ans e a di e en bomba ding ene gies has only been p ope ly done o he case o single
cha ge-exchange [8]. In single cha ge-exchange, he ans e consis s o one neu on (p o on)
pick-up ollowed by a one p o on (neu on) s ipping (o ice e sa) wha means ha can
be sol ed in e ms o 2nd o de Dis o ed Wa e Bo n App oxima ion (DWBA). Fo double
cha ge-exchange we can ha e ans e channels in ol ing ou pa icles, which means he
need o a 4 h o de DWBA. Non-o hogonali y be ween p io and pos ep esen a ion in
asn e gene a es a non-o hogonali y con ibu ion. This e m, oge he wi h simul aneous
and succesi e con ibu ions, con ibu es cohe en ly o he inal o al c oss sec ion. Full 2nd
o de DWBA including simul aneous, succesi e and non-o hogonali y e ms has been ecen ly
ully implemen ed, helping us o calcula e exac c oss sec ions o hese cases, whe eas o 4 h
o de DWBA he e is no implemen a ion ye o he co esponding non-o hogonali ies.
The e o e, ou pu pose is o p elimina y asses he impo ance o he di e en con ibu ions
in o de o s udy he possibili y o ex ac ing he desi ed esponse om he expe imen al da a.
We will es ima e he ans e con ibu ion o he 18O + 40Ca eac ion a 15 MeV/A and we
will compa e wi h he double cha ge-exchange expe imen al da a om [5].
2. Double cha ge-exchange and mul inucleon ans e c oss sec ions
On one hand, we only conside double cha ge exchange as a second o de cha ge exchange, so
ha he o m ac o s needed o he eac ion calcula ion a e hose o he eac ions: 18O+40Ca
→18F+40K and 18F+40K→18Ne+40A . Fo he calcula ion o such o m ac o s we can ely
on a double olding p ocedu e o a esidual nucleon-nucleon in e ac ion and he co esponding
ansi ion densi ies o a ge and p ojec ile.
On he o he hand, co esponding ans e con ibu ions mus be conside ed. The o malism
o mul inucleon ans e in DWBA has been known o se e al decades bu only ecen ly we
ha e s a ed o calcula e second o de DWBA ans e due o i s compu a ional demands. Fo
he case o double cha ge exchange we deal wi h he ans e o wo p o ons and wo neu ons.
Tha would mean he need o a 4 h o de DWBA which has no implemen a ion ye . Since ou
pu pose is o es ima e he o de o magni ude and i s ela i e impo ance wi h espec o he
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cha ge-exchange, we can app oxima e he ull c oss sec ion by he one ob ained conside ing a
second o de DWBA wo-neu on ans e o he g ound s a es o 16O+42Ca ollowed by a second
o de DWBA wo-p o on ans e o he inal p oduc s 18Ne+40A .
We ha e o add he e he possibili y o ha ing one neu on and one p o on ans e ollowed by
a single cha ge exchange and ice e sa. This p ocess is o hi d o de . The e o e, e en hough
i can be agains ou in ui ion o mix wo di e en esponses o nuclei, i could be la ge han
he ull ou h o de ans e .
The s uc u e inpu needed o he ans e a e he di e en o e laps be ween he di e en
a ge -like p oduc s in he di e en ini ial, in e media e and inal si ua ions conside ed. The
same eads o he p ojec ile like ones. Fo he sake o comple eness, hese o e laps should be
p o ided by he same s uc u e calcula ion p o iding ansi ion densi ies o he cha ge exchange
calcula ion. Howe e , hey a e usually app oxima ed by he o e lap ob ained wi h single pa icle
wa e unc ions mul iplied by he co esponding spec oscopic ac o . An al e na i e op ion is o
look o di e en spec oscopic ac o s ex ac ed om expe imen al ans e eac ions on he
conside ed nuclei.
The las ing edien o calcula ing he eac ion c oss sec ion a e he op ical po en ial be ween
he di e en coun e pa s o he ini ial, in e media e, and inal si ua ions. All o hem can
be ob ained again by a double olding p ocedu e wi h he co esponding cen al densi ies o
p ojec ile-like and a ge -like nuclei.
Finally, he o al c oss sec ion is he cohe en sum o all hese con ibu ions. The e o e, we
canno neglec he p ocesses whose c oss sec ions a e small when compu ed sepa a ely. All o
hem in e e e and, h ough his in e e ence, hei inal impac on he o al c oss sec ion can
be la ge han expec ed.
3. P elimina y Resul s
In o de o ackle he 18O + 40Ca eac ion a 15 MeV/A we combine wo p og ams HIDEX [9]
and FRESCO [10]. Wi h HIDEX we calcula e he single cha ge exchange o m ac o by
olding QRPA ansi ion densi ies o he di e en nuclei wi h he Lo e and F aney nucleon-
nucleon in e ac ion [11]. We app oxima e he 18F+40K→18Ne+40A pa by using he same
o m ac o s as in he i s single cha ge exchange, i.e. 18O+40Ca →18F+40K. Howe e ,
including all he cha ge exchange s eng h o all possible mul ipola i ies wi hin FRESCO is e y
demanding compu a ionally, so ha in his p elimina y app oach we ha e cons ain ou sel es
o he mul ipola i y leading o he g ound s a es o he in e media e coun e pa s: 18F(1+) and
40K(4−). Then we inc ease he o al s eng h o his speci ic pa o he o al esponse o he
nuclei in o de o be o he o de o he expe imen al c oss sec ion a ze o deg ees. In his way
he esul should be app oxima e bu s ill ep esen a i e o he s eng h o he double cha ge
exchange p ocess and i s compa ison wi h he compe ing channel emains meaning ul.
We use he same in e ac ion o calcula e he co esponding op ical po en ials. We
include he o m ac o s and op ical po en ials in o FRESCO whe e we can add he di e en
ans e con ibu ions. Fo his las pa , we ely on expe imen ally ex ac ed spec oscopic
ac o s [12, 13, 14, 15] o he di e en cases. Only g ound s a es a e conside ed o e en-e en
o odd-odd nuclei. Fo he odd-e en o e en-odd ones, we conside all he single pa icle le els
in he icini y o he Fe mi ene gy. The e o e, all hese le els p o ide a la ge basis and we only
lack o comple eness in he e en-e en and odd-odd nuclei.
A inal ema k has o be done ega ding he choice o p io o pos in e ac ions o each
s eps. We only conside he successi e pa o he ans e choosing pos in e ac ions o all
he s eps. In o de o ha e he ull ans e c oss sec ion, we will need o conside he di e en
non-o hogonali ies.The ans e leading o he same coun e pa s as DCE is a 4 h o de DWBA
calcula ion. The co esponding non-o hoganli y e ms ha e no been implemen ed so a . A
calcula ion including only succesi e e ms wi h pos in e ac ions, as he calcula ion p esen ed
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he e, should be a good es ima ion and mus each he exac esul i ou basis is inc eased
owa ds comple eness [10].
In o de o assess he ela i e impo ance o pu e ou pa icle ans e , he combina ion
o ans e and a single cha ge exchange and he successi e double cha ge exchange, we ha e
pe o med h ee di e en calcula ion. In he i s one we include all con ibu ions. In he second
one, only cha ge exchange and he combina ion o cha ge exchange and ans e . Finally, in a
hi d calcula ion, only cha ge exchange is included.
We show he p elimina y esul s in able 1. When only double cha ge exchange is conside ed,
we ge a di e en ial c oss sec ion o 18.3 µb/s a ze o deg ees. This alue is an 8% la ge han
he calcula ion ha includes all possible compe ing channels. This las calcula ion is en i led o
be he mos co ec one and he e o e his 8% can be unde s ood as he le el o accu acy ound
when neglec ing he e ec o ans e . Howe e , i we conside he double cha ge exchange in
combina ion wi h one-neu on and one-p o on ans e channels, he di e ence wi h espec o
he ull calcula ion is educed o less han a 5%.
Table 1. P elimina y calcula ions o he di e en ial c oss sec ion a ze o deg ees and he o al
c oss sec ion o he di e en p ocesses conside ed.
P ocesses conside ed dσ
dΩ(0) (µb/s ) In eg a ed σ(µb)
DCE only 18.3 0.060
DCE and (np ans e + SCE) 16.2 0.051
DCE and all ans e s conside ed 17.0 0.054
Expe imen al [5] 11.1 0.072
This educed di e ence is only p esen in he case o he di e en ial c oss sec ion a ze o
deg ees. The angula dis ibu ion also changes depending on he p ocesses conside ed. In ac ,
he esul s o he o al in eg a ed c oss sec ions show a la ge di e ence as can also be ound
in able 1.
4. Conclusions
We ha e s udied he double cha ge exchange eac ion 18O + 40Ca→18Ne+40A a 15 MeV/A
measu ed a he LNS-INFN [5] ocusing in he ela i e impo ance o he di e en compe ing
channels, i.e. double cha ge exchange and he di e en possible ans e combina ions leading
o he same inal nuclei.
We ha e ound ha double cha ge-exchange is he leading p ocess since he e is only a
di e ence o an 8% be ween he di e en ial c oss sec ion a ze o deg ees calcula ed including
all p ocesses conside ed and he one calcula ed by conside ing only he double cha ge-exchange.
This esul was as expec ed acco ding o he ac ha his p ocess is he lowes o de one
conside ed.
Among he p ocesses in ol ing ans e o pa icles, he combina ions o one single cha ge
exchange, one p o on s ipping and one neu on pick up is he ollowing in impo ance.
Conside ing his p ocess and he double cha ge-exchange we ob ain a di e en ial c oss sec ion
a ze o deg ees jus a 5% di e en om he one ob ained including all p ocesses.
Finally, he 4 h o de mul inucleon ans e is he lowes in impo ance. This is impo an
since he e is no a comple e de i a ion and implemen a ion o he co esponding non-
o hogonali y e ms needed o p ope ly calcula e his con ibu ion. This is also consis en wi h
wha ound o he 20Ne + 116Cd eac ion [16] whe e di e en calcula ions o he ans e o
wo neu on and wo p o ons p oduce s ongly supp essed c oss sec ions.
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The combina ions o one single cha ge exchange, one p o on s ipping and one neu on pick
up is a hi d o de p ocess. In o de o do a ull DWBA calcula ion one has o include non-
o hogonali y e ms o he pa ha includes ans e . Howe e , hese non-o hogonali ies a e
pa allel o hose o he second o de p ocess and i s de i a ion should be much simple han
hose o he 4 h o de ans e .
In any case, hese conclusions a e based on p elimina y, no comple e, calcula ions which
should be jus ep esen a i e o he o de o magni ude. Fu he in es iga ions a e demanded
in o de o co obo a e hese p elimina y esul s. Mo eo e , a ull de i a ion o he hi d o de
p ocess a ising om he combina ion o ans e and cha ge exchange could be o g ea in e es
in o de o imp o e accu acy when compa ing ou s uc u e models o neu inoless double-
be a decay candida es wi h he double cha ge-exchange eac ion expe imen al da a. Ano he
issue o in es iga e is whe he he choice o he hea y ion could educe e en mo e his ans e
con ibu ion. As shown in [17], he c oss sec ion o ans e o a pa icle depends o he
alignmen o i s spin wi h i s angula momen um in he ini ial and inal occupied o bi s. This
ea u e is no seen in ans e wi h ligh ions since he pa icles ans e ed a e ini ially in
s−o bi s. Howe e , he ele ance o he ans e can be e y di e en i we use a hea y ion wi h
alence neu ons and p o ons occupying a spin-aligned o a spin-an ialigned o bi .
Acknowledgmen s
The esea ch leading o hese esul s ecei ed unding om Spanish Minis e io de Econom´ıa y
Compe i i idad and FEDER unds unde P ojec No. FIS2014-53448-C2-1-P, by he Ayudas a
Consolidaci´on de G upos om Jun a de Andaluc´ıa, and by he Eu opean Union’s Ho izon 2020
esea ch and inno a ion p og am unde G an Ag eemen No. 654002.
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